Methane emissions from a Californian landfill, determined from airborne remote sensing and in situ measurements

Abstract

Fugitive emissions from waste disposal sites are important anthropogenic sources of the greenhouse gas methane (CH₄). As a result of the growing world population and the recognition of the need to control greenhouse gas emissions, this anthropogenic source of CH₄ has received much recent attention. However, the accurate assessment of the CH₄ emissions from landfills by modeling and existing measurement techniques is challenging. This is because of inaccurate knowledge of the model parameters and the extent of and limited accessibility to landfill sites. This results in a large uncertainty in our knowledge of the emissions of CH₄ from landfills and waste management. In this study, we present results derived from data collected during the research campaign COMEX (CO₂ and MEthane eXperiment) in late summer 2014 in the Los Angeles (LA) Basin. One objective of COMEX, which comprised aircraft observations of methane by the remote sensing Methane Airborne MAPper (MAMAP) instrument and a Picarro greenhouse gas in situ analyzer, was the quantitative investigation of CH₄ emissions. Enhanced CH₄ concentrations or “CH₄ plumes” were detected downwind of landfills by remote sensing aircraft surveys. Subsequent to each remote sensing survey, the detected plume was sampled within the atmospheric boundary layer by in situ measurements of atmospheric parameters such as wind information and dry gas mixing ratios of CH₄ and carbon dioxide (CO₂) from the same aircraft. This was undertaken to facilitate the independent estimation of the surface fluxes for the validation of the remote sensing estimates. During the COMEX campaign, four landfills in the LA Basin were surveyed. One landfill repeatedly showed a clear emission plume. This landfill, the Olinda Alpha Landfill, was investigated on 4 days during the last week of August and first days of September 2014. Emissions were estimated for all days using a mass balance approach. The derived emissions vary between 11.6 and 17.8 ktCH₄ yr ¯¹ with related uncertainties in the range of 14 to 45 %. The comparison of the remote sensing and in situ based CH₄ emission rate estimates reveals good agreement within the error bars with an average of the absolute differences of around 2.4 ktCH₄ yr ¯¹ (±2.8 ktCH₄ yr ¯¹). The US Environmental Protection Agency (EPA) reported inventory value is 11.5 ktCH₄ yr ¯¹ for 2014, on average 2.8 ktCH₄ yr ¯¹ (±1.6 ktCH₄ yr ¯¹) lower than our estimates acquired in the afternoon in late summer 2014. This difference may in part be explained by a possible leak located on the southwestern slope of the landfill, which we identified in the observations of the Airborne Visible/Infrared Imaging Spectrometer – Next Generation (AVIRIS-NG) instrument, flown contemporaneously aboard a second aircraft on 1 day.